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geez... that's a toughie... since he has dirt on his face and has the lorien cape on, I'd say that it's probably a scene in TTT, and before his capture in the orc tower in mordor... and he's looking a little depressed, so maybe the scene where Faramir captures him... i don't know...
That's what I was thinking, but I was looking for that scene and couldn't find it... hmm
Thanks for your help!